Electronic State Spectroscopy Of Acetaldehyde, CH3CHO, By High ...
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Download Free PDFElectronic state spectroscopy of acetaldehyde, CH3CHO, by high-resolution VUV photo-absorptionNigel Mason2003, Chemical Physics Letters
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Acetic acid electronic state spectroscopy by high-resolution vacuum ultraviolet photo-absorption, electron impact, He (I) photoelectron spectroscopy and ab initio calculationsDenis DuflotElectronic state spectroscopy of CH3COOH has been investigated using Vacuum UltraViolet (VUV) photo-absorption spectroscopy in the energy range 3.5–10.6eV. The availability of a high-resolution photon beam (∼0.075nm) has allowed detailed analysis of the vibrational progressions and allowed us to propose, for the first time, new assignments for several Rydberg series. Excited states located in the 10–14eV region have been studied
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downloadDownload free PDFView PDFchevron_rightTropospheric Photolysis Rates of the Acetaldehyde Isotopologues CD3CHO and CD3CDO Relative to CH3CHO Measured at the European Photoreactor Facilityclaus nielsenThe journal of physical chemistry. A, 2015
Acetaldehyde is a hazardous pollutant found in indoor and ambient air. Acetaldehyde photolysis is pressure- and wavelength-dependent with three distinct product channels. In this study, the photolysis rates of CH3CHO, CD3CDO, and CD3CHO are studied in natural tropospheric conditions using long path FTIR spectroscopy, at the European Photoreactor Facility (EUPHORE) in Valencia, Spain. The average relative photolysis rate as an average of four experiments for the fully deuterated isotopologue is jCH3CHO/jCD3CDO = 1.75 ± 0.04, and as a result of a single experiment jCH3CHO/jCD3CHO = 1.10 ± 0.10. These results, combined with our previous determination of jCH3CHO/jCH3CDO = 1.26 ± 0.03, provide mechanistic insight into the photodissociation dynamics of the photoexcited species. Despite the extensive isotopic scrambling in photoexcited acetaldehyde that has recently been reported, the position of the substitution has a clear effect on the relative photolysis rates.
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