Visible Light-driven CO2 Reduction With A Ru Polypyridyl Complex ...

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From the journal:

Chemical Communications

Visible light-driven CO2 reduction with a Ru polypyridyl complex bearing an N-heterocyclic carbene moiety†

Taito Watanabe, a Yutaka Saga,*ab Kento Kosugi, a Hikaru Iwami,a Mio Kondo *abc and Shigeyuki Masaoka *ab Author affiliations

* Corresponding authors

a Department of Applied Chemistry, Graduate School of Engineering, Osaka University, 2-1 Yamadaoka, Suita, Osaka 565-0871, Japan E-mail: [email protected], [email protected], [email protected]

b Innovative Catalysis Science Division, Institute for Open and Transdisciplinary Research Initiatives (ICS-OTRI), Osaka University, Suita, Osaka 565-0871, Japan

c PRESTO, Japan Science and Technology Agency (JST), 4-1-4 Honcho, Kawaguchi, Saitama 332-0012, Japan

Abstract

A novel Ru polypyridyl complex with an N-heterocyclic carbene ligand was successfully synthesised and characterised. The complex exhibited an intense absorption band in the visible-light region derived from the strong electron-donating character of the carbene ligand, and efficiently catalysed the visible light-driven CO2 reduction with the reaction rate of 36.7 h−1.

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Supplementary files

• Supplementary information PDF (1580K)
• Crystal structure data CIF (131K)

Article information

DOI https://doi.org/10.1039/D2CC00657J Article type Communication Submitted 01 Feb 2022 Accepted 15 Mar 2022 First published 15 Mar 2022

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Chem. Commun., 2022,58, 5229-5232 BibTex EndNote MEDLINE ProCite ReferenceManager RefWorks RIS

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Visible light-driven CO2 reduction with a Ru polypyridyl complex bearing an N-heterocyclic carbene moiety

T. Watanabe, Y. Saga, K. Kosugi, H. Iwami, M. Kondo and S. Masaoka, Chem. Commun., 2022, 58, 5229 DOI: 10.1039/D2CC00657J

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