Towards Validation Of Ammonia (NH 3 ) Measurements From The IASI ...
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M. Van Damme
CORRESPONDING AUTHOR martin.van.damme@ulb.ac.be https://orcid.org/0000-0003-1752-0558 Spectroscopie de l'atmosphère, Chimie Quantique et Photophysique, Université Libre de Bruxelles, Brussels, Belgium Cluster Earth and Climate, Department of Earth Sciences, Vrije Universiteit Amsterdam, Amsterdam, the NetherlandsL. Clarisse
https://orcid.org/0000-0002-8805-2141 Spectroscopie de l'atmosphère, Chimie Quantique et Photophysique, Université Libre de Bruxelles, Brussels, BelgiumE. Dammers
https://orcid.org/0000-0003-0128-8205 Cluster Earth and Climate, Department of Earth Sciences, Vrije Universiteit Amsterdam, Amsterdam, the NetherlandsX. Liu
College of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaJ. B. Nowak
https://orcid.org/0000-0002-5697-9807 Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, Colorado, USA Chemical Sciences Division, Earth System Research Laboratory, NOAA, Boulder, Colorado, USA now at: Aerodyne Research, Inc., Billerica, MA, USAC. Clerbaux
Spectroscopie de l'atmosphère, Chimie Quantique et Photophysique, Université Libre de Bruxelles, Brussels, Belgium UPMC; Université Versailles St. Quentin; CNRS/INSU, LATMOS-IPSL, Paris, FranceC. R. Flechard
https://orcid.org/0000-0002-5954-9925 INRA, Agrocampus Ouest, UMR 1069 SAS, Rennes, FranceC. Galy-Lacaux
Laboratoire d'Aérologie, UMR 5560, Université Paul-Sabatier (UPS) and CNRS, Toulouse, FranceW. Xu
College of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaJ. A. Neuman
https://orcid.org/0000-0002-3986-1727 Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, Colorado, USA Chemical Sciences Division, Earth System Research Laboratory, NOAA, Boulder, Colorado, USAY. S. Tang
Centre for Ecology and Hydrology, Edinburgh Research Station, Bush Estate, Penicuik, Midlothian EH26 0QB, UKM. A. Sutton
https://orcid.org/0000-0002-1342-2072 Centre for Ecology and Hydrology, Edinburgh Research Station, Bush Estate, Penicuik, Midlothian EH26 0QB, UKJ. W. Erisman
Cluster Earth and Climate, Department of Earth Sciences, Vrije Universiteit Amsterdam, Amsterdam, the Netherlands Louis Bolk Institute, Driebergen, the NetherlandsP. F. Coheur
Spectroscopie de l'atmosphère, Chimie Quantique et Photophysique, Université Libre de Bruxelles, Brussels, BelgiumAbstract. Limited availability of ammonia (NH3) observations is currently a barrier for effective monitoring of the nitrogen cycle. It prevents a full understanding of the atmospheric processes in which this trace gas is involved and therefore impedes determining its related budgets. Since the end of 2007, the Infrared Atmospheric Sounding Interferometer (IASI) satellite has been observing NH3 from space at a high spatio-temporal resolution. This valuable data set, already used by models, still needs validation. We present here a first attempt to validate IASI-NH3 measurements using existing independent ground-based and airborne data sets. The yearly distributions reveal similar patterns between ground-based and space-borne observations and highlight the scarcity of local NH3 measurements as well as their spatial heterogeneity and lack of representativity. By comparison with monthly resolved data sets in Europe, China and Africa, we show that IASI-NH3 observations are in fair agreement, but they are characterized by a smaller variation in concentrations. The use of hourly and airborne data sets to compare with IASI individual observations allows investigations of the impact of averaging as well as the representativity of independent observations for the satellite footprint. The importance of considering the latter and the added value of densely located airborne measurements at various altitudes to validate IASI-NH3 columns are discussed. Perspectives and guidelines for future validation work on NH3 satellite observations are presented.
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